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Anomalous Diffusion in
Anisotropic Media
Inauguraldissertation zur Erlangung der Doktorwur¨ de
der Fakult¨ at fur¨ Chemie, Pharmazie und Geowissenschaften
der Albert-Ludwigs-Universit¨at
Freiburg im Breisgau
vorgelegt von
Felix Kleinschmidt
aus Freiburg im Breisgau
5. April 2005”Il faut avoir ´etudi´e beaucoup pour savoir peu.”
Montesquieu (1689-1755)
Pens´ees, Nr. 1116
Œuvres compl`etes, Paris 1950Vorsitzender des Promotionsausschusses: Prof. Dr. G. Schulz
Dekan: Prof. Dr. H. Hillebrecht
Referentin: Prof. Dr. C. Schmidt
Korreferent: Prof. Dr. H. Finkelmann
Betreuerin der Arbeit: Prof. Dr. C. Schmidt
Tag der mundlic¨ hen Prufung:¨ 09.05.2005
Die vorliegende Arbeit entstand in der Zeit von April 2001 bis April 2005 am
Institut fur¨ Makromolekulare Chemie der Albert-Ludwigs-Universit¨ at Freiburg
im Breisgau.Publications and Presentations
Publications
Kay Saalw¨ achter, Felix Kleinschmidt and Jens-Uwe Sommer, Swelling Hetero-
geneities in End-Linked Model Networks: A Combined Proton Multiple-Quantum
NMR and Computer Simulation Study, Macromolecules 2004, 37, 8556-8568
Felix Kleinschmidt, Markus Hickl, Claudia Schmidt and Heino Finkelmann: Smec-
2tic Liquid Single Crystal Hydrogels (LSCH): Hygroelastic and H NMR Diffusion
Measurements, in preparation
Felix Kleinschmidt and Claudia Schmidt: MultilamellarVesiclesfromC E /D O;10 3 2
NMR Line Shape and Pulsed Gradient Diffusion Measurements, in preparation
Scientific Talks
Felix Kleinschmidt, Patrick Becker, Laurence Noirez and Claudia Schmidt: Side-
Chain Liquid Crystal Polymers under Shear Flow, Meeting of the TMR network
’Rheology of Liquid Crystals’, Lisbon / Portugal, 5-8/04/2001
Felix Kleinschmidt and Claudia Schmidt: Diffusion in Anisotropic Media, Meet-
ing of the Collaborative Research Centre (SFB) 428, Waldau, 6-7/12/2001
Felix Kleinschmidt, Markus Hickl and Claudia Schmidt: PGSE-Diffusion Mea-
surements in Anisotropic Hydrogels, Meeting ’Solid State NMR Methods and
Applications in Material Sciences’, Oberjoch, 14-18/07/2002
2Felix Kleinschmidt and Claudia Schmidt: Anisotropic Hydrogels: H PGSE Dif-
fusion Measurements, Liquid Crystal Group Meeting, Paderborn, 11/20022Felix Kleinschmidt and Claudia Schmidt: H NMR in Oriented Liquid Crystals,
Meeting of the Collaborative Research Centre (SFB) 428, Waldau, 28-29/11/2002
2Felix Kleinschmidt and Claudia Schmidt: H PGSE Diffusion Measurement in
Oriented Liquid Crystals, ’NMR Spring Workshop’, Bayreuth, 14-17/02/2003
Felix Kleinschmidt and Claudia Schmidt: Structure of Multilamellar Vesicles,
Meeting of the Collaborative Research Centre (SFB) 428, Waldau, 27-28/11/2003
Felix Kleinschmidt and Claudia Schmidt: Diffusion in Multilamellar Vesicles,
’NMR Spring Workshop’, Wandlitz (Berlin), 02/2004
Felix Kleinschmidt and Claudia Schmidt: MultilamellarVesiclesfromC E /D O;10 3 2
NMR Line Shape and Pulsed Gradient Diffusion Measurements, NMR - Group
Meeting, Darmstadt, 26/7/2004
Felix Kleinschmidt and Claudia Schmidt: MultilamellarVesiclesfromC E /D O;10 3 2
NMR Line Shape and Pulsed Gradient Diffusion Measurements, ’32. Workshop
on Liquid Crystals’ of the German Liquid Crystal Society, Halle, 24-26/03/2004
Poster Presentations
Claudia Schmidt, Felix Kleinschmidt and Daniel Burgemeister: Rheo-NMR and
Diffusion Studies in Liquid Crystals, Meeting of the Magnetic Resonance Spec-
troscopy Division of the German Chemical Society, Bremen, 24-27/09/2002
Felix Kleinschmidt and Kay Saalw¨ achter: NMRCharacterizationandSelf-diffusion
Study of Partially Swollen Polymer Networks, Congress ’Macromolecular Collo-
quium’, Freiburg, 27/02-1/03/2003
Felix Kleinschmidt, Markus Hickl, Heino Finkelmann and Claudia Schmidt: Smec-
2tic Liquid Single Crystal Hydrogels (LSCH): Hygroelastic and H NMR Diffusion
Measurements, ’31. Workshop on Liquid Crystals’ of the German Liquid Crystal
Society, Mainz, 19-21/03/2003
Felix Kleinschmidt and Claudia Schmidt: MultilamellarVesiclesfromC E /D O:10 3 2
NMRLineShapeandPFGDiffusionMeasurements, ’GIDRM XXXIV Italian Na-
tional Congress on Magnetic Resonance’, Porto Conte / Sardinia 21-24/09/2004