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Publié par | friedrich-alexander-universitat_erlangen-nurnberg |
Publié le | 01 janvier 2010 |
Nombre de lectures | 40 |
Poids de l'ouvrage | 11 Mo |
Extrait
Nitrogen Storage and Reduction Model
Catalysts from Ultra‐High Vacuum to
Realistic Pressure Conditions
Nitrogen Storage and Reduction (NSR)
Modellkatalysatoren:
vom Ultrahochvakuum zu realen
Druckverhältnissen
Der Naturwissenschaftlichen Fakultät der
Friedrich-Alexander-Universität Erlangen-Nürnberg
zur Erlangung des Doktorgrades Dr. rer. nat.
vorgelegt von
Master of Science (M.Sc.) Aine Desikusumastuti
aus Jakarta
Als Dissertation genehmigt
durch die Naturwissenschaftliche Fakultät
der Friedrich-Alexander-Universität Erlangen-Nürnberg
Tag der mündlichen Prüfung: 06.04.2010
Vorsitzender der Promotionskommission: Prof. Dr. Eberhard Bänsch
Erstberichterstatter: Prof. Dr. Jörg Libuda
Zweitberichterstatter: Prof. Dr. Hans-Peter Steinrück
Teile diese Arbeit wurden bereits in den folgenden Fachzeitschriften oder als Tagungsbeitrag
veröffentlicht:
Fachzeitschriften:
• A. Desikusumastuti, T. Staudt, H. Grönbeck, J. Libuda, “Identifying surface species by
vibrational spectroscopy: Bridging vs monodentate nitrates”, Journal of Catalysis, 2008,
255, 127‐133.
• A. Desikusumastuti, T. Staudt, M. Happel, M. Laurin, J. Libuda, “Adsorption and
reaction of NO on ordered alumina films and mixed baria‐alumina nanoparticles: 2
Cooperative versus non‐cooperative reaction mechanisms”, Journal of Catalysis, 2008,
260, 315‐328.
• A. Desikusumastuti, M. Laurin, M. Happel, Z. qin, S. Shaikhutdinov, J. Libuda, “Strong
Size Effects in Supported Ionic Nanoparticles: Tailoring the Stability of NO Storage x
Catalysts”, Catal Lett, 2008, 121,:311‐318.
• A. Desikusumastuti, Z. Qin, T. Staudt, M. Happel, Y. Lykhach, M. Laurin, S.
Shaikhutdinov, J. Libuda, “Controlling metal/oxide interaction in bifunctional
nanostructured model catalysts: Pd and BaO on Al O /NiAl(110)”, Surface Science, 2 3
2008, 603, L9‐L13.
• A. Desikusumastuti, T. Staudt, Z. Qin, M. Happel, M. Laurin, Y. Lykhach, S.
Shaikhutdinov, F. Rohr, J. Libuda, “Interaction of NO with Model NSR Catalysts: Metal‐2
Oxide Interaction Controls Initial NO Storage Mechanism”, ChemPhysChem, 2008, 9, x
2191‐2197.
• A. Desikusumastuti, M. Happel, K. Dumbuya, T. Staudt, M. Laurin, J. M. Gottfried, H.‐P.
Steinrück, J. Libuda, “Modeling NO Storage Materials: On the Formation of Surface x
Nitrites and Nitrates and Their Identification by Vibrational Spectroscopy”, J. Phys.
Chem. C, 2008, 112, 6477‐6486.
• T. Staudt, A. Desikusumastuti, M. Happel, E. Vesselli, A. Baraldi, S. Gardonio, S. Lizzit, F.
Rohr, J. Libuda, “Modelling NO storage materials: A high‐resolution photoelectron
spectroscopy study on the interaction of NO with Al O /NiAl(110) and BaO/ 2 3
Al O /NiAl(110)”, J. Phys. Chem. C, 2008,112,9835‐9846. 2 3
• F. Viñes, A. Desikusumastuti, T. Staudt, A. Görling, J. Libuda, K. M. Neyman, “A
combined density‐functional and IRAS study on the interaction of NO with Pd
nanoparticles: identifying new adsorption sites with novel properties”, J. Phys. Chem. C,
2008, 112, 16539‐16549.
• A. Desikusumastuti, Z. Qin, M. Happel, T. Staudt, Y. Lykhach, M. Laurin, F. Rohr, S.
Shaikhutdinov, J. Libuda, “Nitrite and nitrate formation on model NO storage materials: x
on the influence of particle size and composition”, Physical Chemistry Chemical Physics,
2009, 11, 2514—2524.
• A. Desikusumastuti, S. Schernich, M. Happel, M. Sobota, M. Laurin, J. Libuda, “Model
NOx Storage Materials at Realistic NO Pressures”, ChemCatChem, 2009, 1(2), 318‐325. 2
• A. Desikusumastuti, M. Happel, Z. Qin, T. Staudt, Y. Lykhach, M. Laurin, S.
Shaikhutdinov, F. Rohr, J. Libuda, “Particle‐Size‐Dependent Interaction of NO with Pd 2
Nanoparticles Supported on Model NOx Storage Materials”, Journal of Physical
Chemistry C , 2009, 113(22), 9755‐9764.
Tagungsbeitrage:
• A. Desikusumastuti, M. Laurin, J. Libuda, “A novel multi molecular beam/reactor/TR‐
IRAS experiment for microkinetic studies and its application to model NO storage x
catalysts, Deutsche Katalytiker Treffen, 2007, Weimar‐Germany.
• A. Desikusumastuti, J. Libuda, “The interaction of supported BaO nanoparticles with
NO ”, COST WG3, 2007, Erlangen‐Germany. 2
• A. Desikusumastuti, M. Happel, M. Laurin, J. Libuda, “Model systems for NO storage x
catalysts: A multi molecular beam/TR‐IRAS study, Bunsentagung, 2007, Graz‐Austria.
• A. Desikusumastuti, T. Staudt, M. Happel, Z. Qin, S. Shaikhutdinov, J. Libuda, “Particle
size dependent formation and decomposition of barium nitrate nanoparticles on
ordered aluminium oxide films”, COST Annual Meeting, 2007, Berlin‐Germany.
• A. Desikusumastuti, T. Staudt, M. Happel, Z. Qin, S. Shaikhutdinov, J. Libuda,
“Modelling NO Storage and Reduction Catalysis: Particle Size Dependent Formation x
and Decomposition of Barium Nitrate Nanoparticles on Ordered Aluminium Oxide
Films”, Deutsche Katalytiker Treffen, 2008, Weimar‐Germany.
• A. Desikusumastuti, T. Staudt, M. Happel, J. Libuda, “Combined Molecular Beam / TR‐
IRAS Experiments on NO Storage and Reduction Model Catalysts”, Bunsentagung, x
2008, Saarbruecken‐Germany.
• A. Desikusumastuti, T. Staudt, M. Happel, S. Gardonio, S. Lizzit, E. Vesselli, A. Baraldi, Z.
Qin, S. Shaikhutdinov, and J. Libuda, “NO Storage Model Catalyst Studied by STM, x
Time‐Resolved IRAS, Molecular Beams and High‐Resolution PES: On the Interaction of
NO with Alumina Supported BaO Nanoparticles”, European Conference of Surface 2
Science, 2008, Liverpool‐England.
• A. Desikusumastuti, T. Staudt, M. Happel, M. Laurin, J. Libuda, “Adsorption and
Reaction of NO on Ordered Alumina Films and Mixed Baria‐Alumina